Wave-vector analysis of plasmon-assisted distributed nonlinear photoluminescence along Au nanowires

Abstract

We report a quantitative analysis of the wave-vector diagram emitted by nonlinear photoluminescence generated by a tightly focused pulsed laser beam and distributed along Au nanowire via the mediation of surface plasmon polaritons. The nonlinear photoluminescence is locally excited at key locations along the nanowire in order to understand the different contributions constituting the emission pattern measured in a conjugate Fourier plane of the microscope. Polarization-resolved measurements reveal that the nanowire preferentially emits nonlinear photoluminescence polarized transverse to the long axis at close to the detection limit wave vectors with a small azimuthal spread in comparison to the signal polarized along the long axis. We utilize the finite-element method to simulate the observed directional scattering by using localized incoherent sources placed on the nanowire. Simulation results faithfully mimic the directional emission of the nonlinear signal emitted by the different portions of the nanowire.